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Epitranscriptomic Sequencing

tRNA Epitranscriptomic Modification Mapping Solution — From Full-Spectrum Quantification to Single-Base Resolution

tRNA epitranscriptomic modification mapping answers two questions at once: which modifications are present and at what level, and exactly where they sit on each tRNA. Arraystar's solution combines base-resolution tRNA modification sequencing — m7G TRAC-Seq, m3C HAC-Seq, tRNA Modification Seq (m1A, m3C, m1G, m2,2G), and tRNA Charging Seq — with full-spectrum LC-MS quantification of 55 nucleoside modifications, for quantitative, position-resolved tRNA modification profiling.

Sample-to-data services · Chemical-specific methods with quantitative stoichiometry assessment

Overview

Two complementary technical routes for quantitative tRNA modification mapping

tRNAs undergo by far the greatest number of, and the most chemically diverse, post-transcriptional modifications. These modifications are critical for all core aspects of tRNA function, such as folding, stability, and decoding [1]. Defects in tRNA modifications and modification enzymes are linked with human diseases such as cancers, diabetes, neurological syndromes, cardiac conditions, and mitochondrial-linked disorders [3]. Studying tRNA modification is perhaps just as important as tRNA expression profiling.

Reliable modification mapping needs two complementary layers of evidence. Base-resolution sequencing localizes individual modifications on specific tRNAs: m7G TRAC-Seq uses reductive cleavage at m7G; m3C HAC-Seq uses hydrazine-aniline cleavage at m3C; tRNA Modification Seq compares demethylase-treated and untreated tRNAs to identify m1A, m3C, m1G, and m2,2G sites; and tRNA Charging Seq detects modification-induced misincorporation during reverse transcription and simultaneously profiles tRNA expression and charging. Full-spectrum quantification (LC-MS) hydrolyzes tRNAs into single nucleosides and simultaneously profiles 55 nucleoside modifications from total RNA, delivering the global modification profile of the sample.

What is tRNA epitranscriptomic modification mapping?

tRNA epitranscriptomic modification mapping identifies and quantifies post-transcriptional modifications on transfer RNAs, either globally as nucleoside profiles (LC-MS) or at precise base positions on individual tRNAs (TRAC-Seq, HAC-Seq, Modification Seq, tRNA Charging Seq), linking modification status to tRNA function and disease.

Service at a Glance

Five tRNA modification mapping services — combine them for integrated epitranscriptomic studies

Service NameModification TargetsResolutionPrice
m7G TRAC-Seq m7G Single-nucleotide
m3C HAC-Seq m3C Single-nucleotide
tRNA Modification Seq – m1A, m3C, m1G, m2,2G m1A, m3C, m1G, m2,2G Single-base
tRNA Charging Seq Broad modification coverage (e.g. m1A, m1G, m3C, acp3U) + tRNA expression & charging Single-nucleotide (predicted)
LC-MS Based tRNA Modification Analysis 55 nucleoside modifications (global profile) Nucleoside-level quantification

Benefits

Why researchers choose Arraystar for tRNA modification mapping

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Full-Spectrum & Base-Resolution Coverage

LC-MS simultaneously profiles 55 nucleoside modifications from total RNA, while sequencing methods map individual modifications at single-base resolution on specific tRNAs.

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Chemical Specificity

TRAC-Seq and HAC-Seq rely on highly specific chemical reactions rather than antibody affinity, eliminating background from non-specific binding and enabling quantitative stoichiometry assessment.

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Multi-Modification in One Assay

tRNA Modification Seq simultaneously detects and quantifies m1A, m3C, m1G, and m2,2G modifications at single-base resolution by comparing demethylase-treated and untreated tRNAs.

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Simultaneous tRNA Profiles

tRNA Charging Seq profiles tRNA expression, tRNA modifications, and tRNA charging at once, with broad modification coverage (e.g. m1A, m1G, m3C, acp3U) predicted at single-nucleotide resolution.

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Sample-to-Data Service

Full-service workflows from sample QC through tRNA isolation, library preparation or nucleoside analysis, sequencing or LC-MS/MS acquisition, to comprehensive bioinformatics and report.

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Integrated tRNA Solutions

All services work well together with Arraystar's broad tRNA research technologies — tRNA-seq, tRF&tiRNA-Seq, PCR arrays, and rtStar™ pretreatment kits — for integrated studies.

Background

tRNA modifications — chemically diverse marks that control tRNA function and disease

tRNAs are the fundamental component of mRNA decoding and protein translation. tRNAs undergo by far the greatest number of and the most chemically diverse post-transcriptional modifications, which are critical for all core aspects of tRNA function, such as folding, stability, and decoding [1]. Typically, modifications in the main body of tRNA are crucial for tRNA structure folding, stability, rigidity, and flexibility, whereas modifications in the anticodon loop affect decoding by open loop structure, codon-anticodon pairing, wobbling, and preventing translational frameshifts. Additionally, modified nucleosides serve as identity determinants for aminoacyl-tRNA synthetase for extra amino acid recognition accuracy [2]. In general, hypomodified tRNAs are targeted for degradation.

Defects in tRNA modifications and modification enzymes are linked with human diseases such as cancers, diabetes, neurological syndromes, cardiac conditions, and mitochondrial-linked disorders (Fig. 1) [3]. m3C at position 32 of the anticodon loop maintains tRNA structure, decoding accuracy, and translation efficiency; dysregulation of m3C-related enzymes and tRNA m3C modifications has been associated with tumor progression and metastasis in cancers such as hepatocellular carcinoma and breast cancer, as well as neurological and mitochondrial disorders. m7G at position 46 in the variable loop, deposited by the METTL1/WDR4 complex, maintains tRNA structural integrity and enhances translation of codon-enriched mRNAs; METTL1 overexpression drives tumorigenesis in leukemia, glioblastoma, cholangiocarcinoma, and lung cancer. Beyond abundance, tRNA expression and charging — the aminoacylation state that determines translation activity — complete the functional picture that epitranscriptomic mapping must resolve (Fig. 2).

Figure 1. tRNA modifications in human diseases
Figure 1. tRNA modifications in human diseases. Defects in tRNA modifications and modification enzymes are linked with cancers, diabetes, neurological syndromes, cardiac conditions, and mitochondrial-linked disorders.
Figure 2. tRNA expression, tRNA modification, and tRNA charging in translation regulation
Figure 2. (A) tRNA expression on translation efficiency and mRNA stability. When an mRNA is well supplied with optimal codon tRNAs, the ribosomes progress fast and the translation is at high efficiency. When an mRNA is limitedly supplied with non-optimal codon tRNAs, the ribosomes progress slowly and the translation is at low efficiency. When mRNA is translated slowly, Dhh1 RNA helicase dissociates ribosomes from the mRNA, causing the mRNA to decay. (B) tRNA modification on translation efficiency and mRNA stability. Here, m5C modification in the tRNA anticodon increases ribosome progression speed, protein translation efficiency, and mRNA stability. The increased RPL22A protein, for example, renders the cells more resistant to reactive oxygen species (ROS). (C) tRNA charging on translation. Increased tRNA charging in cells cultured with the supplemented amino acid has higher protein translation with the optimal mRNA.

Background References

  1. Kirchner S, et al. Emerging roles of tRNA in adaptive translation, signalling dynamics and disease. Nature Reviews Genetics, 2015. PMID: 25534324
  2. El Yacoubi B, et al. Biosynthesis and function of posttranscriptional modifications of transfer RNAs. Annual Review of Genetics, 2012. PMID: 22905870
  3. Torres AG, et al. Role of tRNA modifications in human diseases. Trends in Molecular Medicine, 2014. PMID: 24581449
  4. Orellana EA, et al. tRNA dysregulation and disease. Nature Reviews Genetics, 2022. PMID: 35681060

Solution Workflow — Building Your Evidence Chain

From total RNA to a quantitative, position-resolved tRNA modification map

1

Sample & RNA QC

Total RNA quality and quantity assessment before the project proceeds, with small-RNA-retaining purification.

2

Global Modification Quantification

LC-MS route: tRNA isolation from total RNA, complete hydrolysis and dephosphorylation to single nucleosides, and UHPLC-MS/MS quantification of 55 nucleoside modifications.

3

Base-Resolution Modification Mapping

Select the sequencing method by target: m7G TRAC-Seq (reductive cleavage), m3C HAC-Seq (hydrazine-aniline cleavage), tRNA Modification Seq (demethylase ± comparison), or tRNA Charging Seq (reverse-transcription misincorporation).

4

Bioinformatics

Differential modification analysis, IGV read alignments for site identification, sequence motif analysis, and volcano plots.

5

Integrative Interpretation

Combine global and positional modification data, and cross-reference with tRNA expression, charging, and tRF/tiRNA profiles.

Workflow of Arraystar LC-MS tRNA Modification Analysis
Figure 3. Workflow of Arraystar LC-MS tRNA Modification Analysis. Total RNA is used as the starting material; the service includes tRNA isolation, complete hydrolysis, and dephosphorylation to prepare single nucleosides for LC-MS/MS quantification.
Workflow of tRNA Modification Seq for m1A, m3C, m1G, and m2,2G
Figure 4. Workflow of tRNA Modification Seq. m1A, m3C, m1G, and m2,2G modifications are identified by their induced misincorporation mutations in reverse transcription compared with demethylase-treated tRNA.
m7G TRAC-Seq workflow
Figure 5. m7G TRAC-Seq workflow. Isolated tRNAs are enzymatically demethylated and treated with NaBH4/aniline to induce reductive cleavage specifically at m7G residues. The 3' cleavage fragments are ligated with a sequencing adaptor at their 5'-ends where the precise modification sites are located; m7G sites and modification levels are identified by cleavage scores.
m3C HAC-Seq workflow
Figure 6. m3C HAC-Seq workflow. Isolated tRNAs were treated with hydrazine and aniline (HAC) to cleave the RNA backbone at m3C sites. To confirm specificity, samples were treated with demethylase prior to HAC (DM-HAC) to remove m3C modifications. Since HAC-generated 5' fragments contain damaged 3' ends that preclude adapter ligation, m3C sites were identified at single-nucleotide resolution by calculating the cleavage ratio.

Bioinformatics & Deliverables

Detailed bioinformatics analyses included in every tRNA modification mapping service

Each service includes detailed bioinformatics analyses to facilitate insights into tRNA modifications in biology, diseases, and biomarker applications. m7G TRAC-Seq delivers m7G sites and modification levels by cleavage scores; m3C HAC-Seq identifies m3C sites at single-nucleotide resolution by cleavage ratio; tRNA Modification Seq analyzes modification sites, methylation levels, and tRNA expression at once; and tRNA Charging Seq provides a wealth of tRNA multi-omics data with common analyses (e.g. differential analyses) and detailed annotations. LC-MS projects report raw and normalized peak data, Total Ion Current chromatograms of nucleosides, and differential modification of nucleosides among samples.

Standard Deliverables

Volcano plot for differentially expressed m7G-tRNAs
Figure 7. Volcano plot for differentially expressed m7G-tRNAs. Differential analysis highlights m7G-modified tRNAs that change between comparison groups.
IGV displays of read alignments around m3C32 sites on different tRNA
Figure 8. IGV displays of read alignments around m3C32 sites on different tRNA. Cleavage-induced read patterns pinpoint modification sites at single-nucleotide resolution.
Sequence motif analysis of m3C-modified tRNAs
Figure 9. Sequence motif analysis of m3C-modified tRNAs. Modification-associated sequence motifs are discovered from mapped m3C sites.
tRNA Modification Heatmap
Figure 10. tRNA Modification Heatmap. Heatmap view of modification profiles across samples for comparative analysis.
Total Ion Current chromatogram of nucleosides
Figure 11. Total Ion Current chromatogram of nucleosides. LC-MS detection of modified nucleosides from hydrolyzed tRNA samples.
Differential modification of nucleosides among samples
Figure 12. Differential modification of nucleosides among samples. Quantitative comparison of nucleoside modification levels across experimental groups.

Research Applications

tRNA modification mapping across biology and disease

Cancer Biology

m7G-modified tRNAs (e.g. Arg-TCT-4-1, Lys-CTT, Val-AAC) drive tumorigenesis in leukemia, glioblastoma, cholangiocarcinoma, and lung cancer (Mol Cell, 2021); m3C dysregulation is associated with tumor progression and metastasis in hepatocellular carcinoma and breast cancer.

Neurological & Mitochondrial Disorders

METTL8-dependent mitochondrial tRNA m3C is indispensable for neural stem cell maintenance (Cell Stem Cell, 2023); DALRD3-dependent modification of tRNA-Arg is crucial for neurological function (Nat Commun, 2020).

Translation Regulation & Cell Fate

m3C32 tRNA modification controls serine codon-biased mRNA translation, cell cycle, and DNA-damage response (Nat Commun, 2024); m7G-modified tRNAs enhance translation efficiency of codon-enriched oncogenic mRNAs.

Stem Cell Self-Renewal & Development

METTL1/WDR4-mediated m7G tRNA methylome is required for embryonic stem cell self-renewal and differentiation (Mol Cell, 2018); METTL6-mediated modification of tRNA-Ser supports pluripotency and tumorigenesis (Sci Adv, 2020).

Metabolic & Cardiovascular Disease

tRNA modification profiles link to diabetes and cardiac conditions; glutamyl-prolyl-tRNA synthetase regulates pro-fibrotic protein synthesis during cardiac fibrosis (Circ Res, 2020); tRNA Charging Seq applications include cardiac fibrosis and cancer drug resistance.

Drug Resistance & Therapeutics

Valine aminoacyl-tRNA synthetase promotes therapy resistance in melanoma (Nat Cell Biol, 2024); dual targeting of m7G tRNA modification and histone acetylation evokes osteosarcoma chemosensitization (Adv Mater, 2025).

Choosing the Right Strategy for Your Study

Method selection depends on your modification targets and the resolution you need

DimensionTRAC-Seq (m7G)HAC-Seq (m3C)tRNA Modification SeqtRNA Charging SeqLC-MS Based tRNA Modification Analysis
Modification targetsm7Gm3Cm1A, m3C, m1G, m2,2GBroad coverage (e.g. m1A, m1G, m3C, acp3U), predicted55 nucleoside modifications (global profile)
ResolutionSingle-nucleotideSingle-nucleotideSingle-baseSingle-nucleotide (predicted)Nucleoside-level quantification
Key principleNaBH4/aniline reductive cleavageHydrazine-aniline cleavageDemethylase-treated comparison (methylation index)Reverse transcription misincorporationHydrolysis + LC-MS/MS of single nucleosides
Additional profilesm7G sites & levelsm3C sites & levelstRNA expressiontRNA expression & chargingGlobal nucleoside modification status
Recommended total RNA> 5 µg*> 5 µg*> 5 µg*> 5 µg*10*–15 µg

Sample Requirements

Official Arraystar sample submission requirements for tRNA modification mapping projects

RNA Amount & Quality

  • Total RNA input: > 5 µg per sample for TRAC-Seq, HAC-Seq, tRNA Modification Seq, and tRNA Charging Seq; 10*–15 µg for LC-MS analysis. Supply twice the recommended minimum to avoid project delays.
  • Purification: TRIzol / RNA precipitation or an RNA isolation kit. Because tRNA is < 200 nt, use a kit specified to retain small RNAs (e.g. Qiagen miRNeasy).
  • Concentration: > 20 ng/µL by Nanodrop; OD260/280 ~2.0 (acceptable 1.7–2.1); OD260/230 > 1.8.
  • Integrity: sharp 18S/28S rRNA bands by gel, or RIN > 7.0 by Bioanalyzer (serum/plasma/exosome/FFPE RNA exempt).
  • DNase treatment: optional for gDNA removal; required if the sample is also used for qPCR.

Shipping Instructions

  • Ship RNA in nuclease-free water (> 20 ng/µL), freeze-dried, or in ethanol; store at −80 °C or in liquid nitrogen.
  • Use nuclease-free certified, screw-cap 1.5 mL microtubes; seal caps with Parafilm; place tubes in a plastic bag.
  • Use 10 kg dry ice as refrigerant; include a signed Project Form in a waterproof bag, separate from samples.
  • Avoid Thursday/Friday drop-offs before weekends or holidays; email the tracking number to your Arraystar representative.
Service / Sample TypeRequirementNotes
TRAC-Seq / HAC-Seq / tRNA Modification Seq> 5 µg total RNA*Recommended minimum for the entire experiment including sample QC
tRNA Charging Seq> 5 µg total RNA*Recommended minimum for the entire experiment including sample QC
LC-MS tRNA Modification Analysis10*–15 µg total RNAtRNA isolation performed from the submitted total RNA
Cultured cells2 × 10⁶ cellsLyse immediately in TRIzol (1 mL per 5–10 × 10⁶ suspension cells or 10 cm² dish); ship on dry ice
Tissue10–25 mgRNAlater (≥10 volumes, 2–8 °C overnight), TRIzol (1 mL per 10–25 mg), or fresh-frozen in liquid nitrogen
Whole blood2–3 mL (0.3 mL/aliquot)Services with pretreatment → use the “With IP or Pretreatment” volumes; ship on dry ice
Plasma / Serum2–5 mL (0.3 mL/aliquot)EDTA or citrate anticoagulant; do NOT use heparin; ship on dry ice

* Recommended minimum amount per sample for the entire experiment in a single attempt, including sample QC; supply twice the recommended minimum to avoid project delays. If the minimum amount is not obtainable, contact support@arraystar.com for special arrangements. Arraystar performs sample QC upon receipt; QC assessment is final. Low amount/quality samples may proceed with consent — data quality and success rate may decline. Shipping address: ATTN: Samples Receiving (Project#______), Arraystar Inc., 9430 Key West Avenue #128, Rockville, MD 20850 USA, Tel: 888-416-6343.

FAQ

Common questions about tRNA epitranscriptomic modification mapping

How do I choose between LC-MS and base-resolution sequencing for tRNA modification analysis?
LC-MS simultaneously quantifies 55 nucleoside modifications from total RNA and characterizes the global modification profile of tRNAs. Sequencing methods then localize individual modifications on specific tRNAs: m7G TRAC-Seq for m7G, m3C HAC-Seq for m3C, tRNA Modification Seq for m1A, m3C, m1G, and m2,2G, and tRNA Charging Seq for broad modification coverage together with tRNA expression and charging profiles.
How does TRAC-Seq detect m7G at single-nucleotide resolution?
TRAC-Seq (tRNA reduction and cleavage sequencing) is a chemical method for single-nucleotide resolution profiling of m7G throughout tRNA transcriptome. Isolated tRNAs are demethylated and treated with NaBH4/aniline to cleave specifically at m7G residues. 3' cleavage fragments are ligated with an adaptor at their 5'-ends, where modification sites are located; m7G sites and levels identified by cleavage scores.
How does HAC-Seq detect m3C?
HAC-Seq (hydrazine-aniline cleavage sequencing) maps tRNA m3C modifications at single-nucleotide resolution. Isolated tRNAs are treated with hydrazine and aniline (HAC) to cleave RNA backbone at m3C sites; samples treated with demethylase prior to HAC (DM-HAC) remove m3C to confirm specificity. Because HAC-generated 5' fragments contain damaged 3' ends that preclude adapter ligation, m3C sites are identified by calculating cleavage ratio.
What is the minimum RNA amount required for these services?
We recommend more than 5 µg of total RNA per sample for m7G TRAC-Seq, m3C HAC-Seq, tRNA Modification Seq, and tRNA Charging Seq, and 10–15 µg for LC-MS based tRNA modification analysis — the official recommended minimum for the entire experiment in a single attempt, including sample QC. Supplying twice the recommended minimum helps avoid project delays.
Can I combine LC-MS quantification with base-resolution sequencing in one project?
Yes. These services work well together within Arraystar's broad portfolio of tRNA research technologies. LC-MS provides the global modification profile of your sample, while sequencing methods map modification sites at base resolution; tRNA Charging Seq additionally reports tRNA expression and charging. Integrative analyses are also available with other Arraystar services, including tRNA-seq, tRF&tiRNA-Seq, and Arraystar small RNA arrays.
What bioinformatics analyses are included?
Detailed bioinformatics analyses are included in each service. Sequencing services deliver differential modification analyses with volcano plots, IGV displays of read alignments for modification site identification, and sequence motif analysis of modified tRNAs. LC-MS projects include raw and normalized peak data, Total Ion Current chromatograms of nucleosides, and differential modification of nucleosides among samples, with publication-ready graphics and visualization.

Selected Publications

Featured Client Publications in tRNA Modification Research

  1. Zhang F, et al. Epitranscriptomic regulation of cortical neurogenesis via Mettl8-dependent mitochondrial tRNA m(3)C modification. Cell Stem Cell, 2023. PMID: 36764294
  2. Cui J, et al. m(3)C32 tRNA modification controls serine codon-biased mRNA translation, cell cycle, and DNA-damage response. Nature Communications, 2024. PMID: 38982125
  3. Lentini JM, et al. DALRD3 encodes a protein mutated in epileptic encephalopathy that targets arginine tRNAs for 3-methylcytosine modification. Nature Communications, 2020. PMID: 32427860
  4. Ignatova VV, et al. METTL6 is a tRNA m(3)C methyltransferase that regulates pluripotency and tumor cell growth. Science Advances, 2020. PMID: 32923617
  5. Lin S, et al. Mettl1/Wdr4-Mediated m(7)G tRNA Methylome Is Required for Normal mRNA Translation and Embryonic Stem Cell Self-Renewal and Differentiation. Molecular Cell, 2018. PMID: 29983320
  6. Orellana EA, et al. METTL1-mediated m(7)G modification of Arg-TCT tRNA drives oncogenic transformation. Molecular Cell, 2021. PMID: 34352207
  7. Dai Z, et al. N(7)-Methylguanosine tRNA modification enhances oncogenic mRNA translation and promotes intrahepatic cholangiocarcinoma progression. Molecular Cell, 2021. PMID: 34352206
  8. Ma J, et al. METTL1/WDR4-mediated m(7)G tRNA modifications and m(7)G codon usage promote mRNA translation and lung cancer progression. Molecular Therapy, 2021. PMID: 34371184
  9. Behrens A, et al. High-resolution quantitative profiling of tRNA abundance and modification status in eukaryotes by tRNA Charging Seq. Molecular Cell, 2021. PMID: 33581077
  10. El-Hachem N, et al. Valine aminoacyl-tRNA synthetase promotes therapy resistance in melanoma. Nature Cell Biology, 2024. PMID: 38849541

Map tRNA Modifications at Full Spectrum and Single-Base Resolution

Arraystar combines full-spectrum LC-MS quantification of 55 nucleoside modifications with single-base resolution tRNA modification sequencing — get a quote and a project design tailored to your modification targets.